Johnny Cash gives James Bond a new sort of soul with "Thunderball," the theme song for the eponymous spy flick. This is the harpoon-laced opening sequence to the 1965 adaptation, with the lyrics of the song describing the film's story.

The song itself is terrific, but it's worth tracking down the DVD and watching Sean Connery do his thing. There's a jet pack involved. [YouTube]

Johnny Cash: ThunderballS